I've been listening to Iron Horse recently ( www.myspace.com/ironhorsebluegrass ) and I was wondering how they would go about creating their harmonies, like what intervals and such they would use.

Any help would be appreciated
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That band is great, I have the cd of modest mouse bluegrass tunes that's really good. Bluegrass usually uses 3-part harmonies, which basically follow the root, 3rd, and 5th intervals.
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